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It is a two-CD set. The first CD collects several rare tracks O'Connor recorded as B-sides, for soundtrack albums or in collaboration with other artists, and the second disc contains a live concert.

The album's title is a modification of Psalm 91, verse 1. This is the same psalm that gave O'Connor's first album, The Lion and the Cobra, its name. The album sold 100,000 copies worldwide.

She Who Dwells in the Secret Place of the Most High Shall Abide Under the Shadow of the Almighty (yeah, it's a mouthful, but at least it's not Fiona Apple's monolith), was reportedly Sinead O' Connor's final album -- it wasn't -- as she seeks another way of life as a spiritual pilgrim, O'Connor delved deep into her rare, B-side, unreleased, and compilation tracks and gives listeners a live album to boot over two discs. Released stateside on Vanguard, this is, despite its disparate nature, one of the most satisfying recordings she's ever delivered -- the previous year's Sean-Nós Nua, her traditional album, was a knockout and perhaps her finest studio moment, but it went unnoticed here because Americans can't seem to forgive O'Connor for exercising her right to free speech (the audience at Bob Dylan's 30th anniversary concert should be especially ashamed). 

The studio sides released on disc one include her collaborations with everyone from Adrian Sherwood to the Asian Dub Foundation to Massive Attack to Roger Eno. Her covers of Dan Penn's "Do Right Woman," Boudleaux Bryant's "Love Hurts," and the B-52's' "Ain't It a Shame" are highly original, deeply moving, and satisfying. Her originals, such as "No Matter How Hard I Try," "Love Is Ours," "This Is a Rebel Song," and "Emma's Song," are eclipsed only by her readings of traditional Gaelic material. Her arrangements and those of her collaborators are top-flight. There are 19 cuts in all on disc one, and not a moribund moment in the bunch.