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Set in Academy City, a city of scientifically advanced superhuman students located western of Tokyo, but in a world where magic is also real. Kamijou Touma 's right hand, the Imagine Breaker, will negate all magic, psychic, or divine powers, but not his own bad luck. One day he finds a young girl hanging on his balcony railing. She turns out to be a nun from the Church of England, and her mind has been implanted with the Index-Librorum-Prohibitorum - all the magical texts the Church has removed from circulation. His encounter with her leads him to meet others from the secret world of science and magic and an adventure with his friends where science and magic collide.

Touma's unusual power places him at the center of conflicts relating magicians and science-based espers in Academy City. As Touma tries to help and protect his friends, he learns the people he knows are not as they appear and begins to attract the attention of magicians and espers alike as they try to unravel the secrets of Academy City and Index.